CMSA Strongly Correlated Quantum Materials and High-Temperature Superconductors Series: Essential Ingredients for Superconductivity in Cupper Oxide Superconductors


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November 6, 2020 12:30 pm - 2:00 pm
via Zoom Video Conferencing

Zhi‐Xun Shen - Stanford University and SLAC National Accelerator Laboratory

High‐temperature superconductivity in cupper oxides, with critical temperature well above what was anticipated by the BCS theory, remains a major unsolved physics problem. The problem is fascinating because it is simultaneously simple ‐ being a single band and 1⁄2 spin system, yet extremely rich ‐ boasting d‐wave superconductivity, pseudogap, spin and charge orders, and strange metal phenomenology. For this reason, cuprates emerge as the most important model system for correlated electrons – stimulating conversations on the physics of Hubbard model, quantum critical point, Planckian metal and beyond. Central to this debate is whether the Hubbard model, which is the natural starting point for the undoped magnetic insulator, contains the essential ingredients for key physics in cuprates. In this talk, I will discuss our photoemission evidence for a multifaceted answer to this question [1‐3]. First, we show results that naturally points to the importance of Coulomb and magnetic interactions, including d‐wave superconducting gap structure [4], exchange energy (J) control of bandwidth in single‐hole dynamics [5]. Second, we evidence effects beyond the Hubbard model, including band dispersion anomalies at known phonon frequencies [6, 7], polaronic spectral lineshape and the emergence of quasiparticle with doping [8]. Third, we show properties likely of hybrid electronic and phononic origin, including the pseudogap [9‐11], and the almost vertical phase boundary near the critical 19% doping [12]. Fourth, we show examples of small q phononic coupling that cooperates with d‐wave superconductivity [13‐15]. Finally, we discuss recent experimental advance in synthesizing and investigating doped one‐dimensional (1D) cuprates [16]. As theoretical calculations of the 1D Hubbard model are reliable, a robust comparison can be carried out. The experiment reveals a near‐neighbor attractive interaction that is an order of magnitude larger than the attraction generated by spin‐superexchange in the Hubbard model. Addition of such an attractive term, likely of phononic origin, into the Hubbard model with canonical parameters provides a quantitative explanation for all important experimental observable: spinon and holon dispersions, and holon‐ holon attraction. Given the structural similarity of the materials, It is likely that an extended two‐dimensional (2D) Hubbard model with such an attractive term, will connect the dots of the above four classes of experimental observables and provide a holistic understanding of cuprates, including the elusive d‐wave superconductivity in 2D Hubbard model.

[1] A. Damascelli, Z. Hussain, and Z.‐X. Shen, Review of Modern Physics, 75, 473 (2003)
[2] M. Hashimoto et al., Nature Physics 10, 483 (2014)
[3] JA Sobota, Y He, ZX Shen ‐ arXiv preprint arXiv:2008.02378, 2020; submitted to Rev. of Mod. Phys.
[4] Z.‐X. Shen et al., Phys. Rev. Lett. 70, 1553 (1993)
[5] B.O. Wells et al., Phys. Rev. Lett. 74, 964 (1995)
[6] A. Lanzara et al., Nature 412, 510 (2001)
[7] T. Cuk et al., Phys. Rev. Lett., 93, 117003 (2004)
[8] K.M. Shen et al., Phys. Rev. Lett., 93, 267002 (2004)
[9] D.M. King et al., J. of Phys. & Chem of Solids 56, 1865 (1995)
[10] D.S. Marshall et al., Phy. Rev. Lett. 76, 484 (1996)
[11] A.G. Loeser et al., Science 273, 325 (1996)
[12] S. Chen et al., Science, 366, 6469 (2019)
[13] T.P. Devereaux, T. Cuk, Z.X. Shen, N. Nagaosa, Phys. Rev. Lett., 93, 117004 (2004)
[14] S. Johnston et al., Phys. Rev. Lett. 108, 166404 (2012)
[15] Yu He et al., Science, 362, 62 (Oct. 2018)
[16] Z. Chen, Y. Wang et al., preprint, 2020